Improving Air Quality in the UK: Developing a mass-closure model for particulate matter
Submitting Institution
University of BirminghamUnit of Assessment
Earth Systems and Environmental SciencesSummary Impact Type
EnvironmentalResearch Subject Area(s)
Chemical Sciences: Analytical Chemistry, Other Chemical Sciences
Engineering: Environmental Engineering
Summary of the impact
Particulate Matter is now recognised as the air pollutant with the
greatest public health impact, estimated to cost up to £8.5-20.2 billion
per annum (in 2005).Roy Harrison has engaged closely with UK policy-makers
for decades. This impact case study focuses specifically on the take-up of
PM mass-closure techniques developed by Harrison's group into a UK
policy-making tool called Pollution Climate Mapping (PCM). Work by the
Harrison group forms the basis of the component dealing with airborne
particles in the PCM model used by Defra. The work described in this case
study has economic impact in the form of costs avoided by the UK
national, devolved and local governments (reallocation of public budgets
away from expensive air pollution monitoring and avoidance of EU financial
penalties), public policy impact in the form of cost-effective
delivery of air pollution mapping, and environmental impact in the
form of traceable inclusion of research in government policies for air
quality improvement.
Underpinning research
Development of cost-effective abatement strategies for airborne
particulate matter depends critically upon developing a sound quantitative
understanding of the contribution of different sources to particulate
matter concentrations measured in the atmosphere. This requires advanced
receptor modelling and Harrison's group has led this activity in the UK
over the past three decades. The case study team comprise: Professor Roy
Harrison, Queen Elizabeth II Birmingham Centenary Professor of
Environmental Health; Dr Royston Lawrence (Research Fellow, 1999 - 2005);
Dr Jianxin Yin (Research Fellow 2001 — ); and Dr Alan Jones (Research
Fellow, 2000 —).
A particular focus of the research has been how aerosol composition can
be used to infer sources of particles. This has included research on "mass
closure", which reconciles the measured total mass concentration with
measurements of individual or groups of chemical compounds that reside in
the aerosol. Mass closure is an essential step in characterisation of the
aerosol and hence the contribution of various sources (e.g., traffic,
industry, dust resuspension, and natural sources) to the total measured
aerosol signal. The group have successfully applied their mass closure and
source apportionment techniques to measurements of airborne particles in
the UK and have contributed to a number of international assessments.
Insights into particulate matter composition as an indicator of source
were gained in the two campaigns of the PUMA consortium project (led by
Harrison) in Birmingham in 1999 and 2000 (Harrison et al., 2006). These
results were used to inform the design of measurements and analysis of
data from the DfT-funded TRAMAQ project, which led to the development of
the Pragmatic Mass Closure Model (Harrison et al., 2003) which was a
parsimonious empirical model which accounted very closely for the measured
mass of airborne particulate matter through measurement of a small suite
of chemical components. With funding from Defra, the Pragmatic Mass
Closure Model was applied to different size fractions of particles (PM1.0,
PM2.5 and PM10) at roadside, urban background and rural sites in the UK,
and its applicability across the full range of particle sizes and
composition was demonstrated (Yin and Harrison 2008). Insights gained from
the measurement campaigns were also used to inform chemistry-transport
modelling activity (Abdalmogith et al., 2006) and elements of each of
these papers were taken up by John Stedman and his colleagues in AEA
Technology (now Ricardo-AEA) and used in the formulation, parameterisation
and development of the Pollution Climate Mapping (PCM) Model.
References to the research
[The three references which best indicate the quality of research
underpinning the case are 1, 4 and 6]
1. A Pragmatic Mass Closure Model for Airborne Particulate Matter at
Urban Background and Roadside Sites, R.M. Harrison, A.M. Jones and R.G.
Lawrence, Atmos. Environ., 37,4927-4933 (2003). DOI:
10.1016/j.atmosenv.2003.08.025
2. Major Component Composition of PM10 and PM2.5 from Roadside and Urban
Background Sites, R.M. Harrison, A.M. Jones and R.G. Lawrence, Atmos.
Environ., 38, 4531-4538 (2004). DOI: 10.1016/j.atmosenv.2004.05.022
3. Particulate Sulphate and Nitrate in Southern England and Northern
Ireland during 2002/3 and its Formation in a Photochemical Trajectory
Model, S.S. Abdalmogith, R.M. Harrison and R.G. Derwent, Sci. Tot.
Environ., 368, 769-780 (2006). DOI: 10.1016/j.scitotenv.2006.02.047
4. Measurement and Modelling of Air Pollution and Atmospheric Chemistry
in the UK West Midlands Conurbation: Overview of the PUMA Consortium
Project, R.M. Harrison, J. Yin, R.M. Tilling, X. Cai, P.W. Seakins, J.R.
Hopkins, D.L. Lansley, A.C. Lewis, M.C. Hunter, D.E. Heard, L.J.
Carpenter, D.J. Creasey, J.D. Lee, M.J. Pilling, N. Carslaw, K.M.
Emmerson, A. Redington, R.G. Derwent, D. Ryall, G. Mills and S.A. Penkett,
Sci. Tot. Environ., 360, 5-25 (2006). DOI: 10.1016/j.scitotenv.2005.08.053
5. Pragmatic Mass Closure Study for PM1.0, PM2.5 and PM10 at Roadside,
Urban Background and Rural Sites, J. Yin and R.M. Harrison, Atmos.
Environ., 42, 980-988 (2008). DOI:10.1016/j.atmosenv.2007.10.005
6. Source Apportionment of Fine Particles at Urban Background and Rural
Sites in the UK Atmosphere, J. Yin, R.M. Harrison, Q. Chen, A. Rutter and
J.J. Schauer, Atmos. Environ.,44, 841-851 (2010). DOI:
10.1016/j.atmosenv.2009.11.026
Details of the impact
Particulate Matter (PM-PM10 and PM2.5) is now recognised as the air
pollutant with the greatest public health impact. The continuing
importance of this issue was underlined in the UK's Air Quality Strategy
(published in 2007) [source 1] which said that the estimated effect of
man-made PM pollution in 2005 would be expected to reduce life expectancy
averaged over the whole population of the UK by up to about 7-8 months.
This health impact in 2005 was estimated to cost up to £8.5-20.2 billion
per annum. The assessment estimated that if no further measures in
addition to those already agreed at the time were implemented, man-made PM
air pollution in the UK would continue to reduce average life expectancy
by up to about 5.5 months even by 2020. This health impact in 2020 was
estimated to cost up to £6.2-14.7 billion per annum (vol. 1 p42 and vol. 2
pp42-43) [source 1].
Roy Harrison has engaged closely with UK policy-makers for decades. Until
recently he served as a member of Defra Science Advisory Council [2009 -
2012], and is currently a member of the Department of Health Committee on
the Medical Effects of Air Pollutants and the Defra Air Quality Expert
Group. He has previously chaired the Quality of Urban Air Review Group
[1991 - 1997] and the Airborne Particles Expert Group [1998 - 1999] for
Defra's predecessor departments and was a member of Defra's Advisory
Committee on Hazardous Substances [2001 - 2006]. He led the preparation of
the Second Report of the Quality of Urban Air Review Group (1993) which
warned of the problems associated with particulate matter and NOx
emissions from diesel vehicles.
This impact case study focuses specifically on the take-up of PM
mass-closure techniques developed by Harrison's group into a UK
policy-making tool called Pollution Climate Mapping.
Pollution Climate Mapping
The results from this research have been used extensively to inform the
Pollution Climate Mapping (PCM) model used by the Department for
Environment, Food and Rural Affairs (Defra) and the Devolved
Administrations to predict future concentrations of airborne pollutants
and to evaluate and compare abatement strategies. (Note: reference to
Defra, below, should always be taken to include the Devolved
Administrations).
The PCM model is currently the sole model chosen by Defra to help meet EU
Air Quality Directive (2008/50/EC) requirements to report on the
concentrations of particular pollutants in the atmosphere at ground level
(Williams et al., 2011) [source 2]. The PCM model is used for compliance
reporting as a substitute for widespread monitoring; it is vital,
therefore, that its components have a strong evidence base (vide section
3, above, for the PM component of PCM). PCM is also used for scenario
assessment and population exposure calculations to assist policy
developments.
The PCM models are run by Ricardo-AEA on behalf of Defra. Work by the
Harrison group forms the basis of the component of the model dealing with
airborne particles used by scientists at AEA [sources 3 & 4]. Annual
reports to Defra are published by AEA summarising the results of UK
modelling under the Air Quality Directive (2008/50/EC) [sources 5 &
6]. The model for particulate matter is described in detail in the report
for 2010 (AEA, 2011) [source 6], describing the model for particulate
matter on pages 70-86. It is clear from the model description that the
fundamental formulation is based upon the receptor modelling work and
Pragmatic Mass Closure Model developed at the University of Birmingham and
the coefficients (e.g. Table 2, page 80 of AEA, 2011) derive directly from
the work of the Harrison group as reported in Abdalmogith et al. (2006),
Harrison et al. (2006) and the report to Defra cited by AEA (2011) as
Harrison and Yin (2006) which was published as Yin and Harrison (2008).
A number of benefits have flowed from use of the model:
- Under article 7 of Directive 2008/50/EC, the number of monitoring
stations may be reduced by 50% if high quality modelling is used to
estimate pollution levels in other locations. The total Defra operational
budget for automatic air quality monitoring in the UK is £3.1M per annum,
of which a substantial portion relates to particulate matter. The capital
cost of instruments installed is of the order of £3M.
- The model output forms the basis of background maps of air quality
across the UK produced by AEA on behalf of Defra (http://laqm.defra.gov.uk/review-and-assessment/tools/background-maps.html).
These maps are considered the definitive information source on air quality
used in all environmental impact assessments within planning applications,
by local government in their air quality assessments and the Planning
Inspectorate in Public Inquiries. Planning applications worth many
billions of pounds each year depend upon the background air quality maps
in their environmental assessments.
- The PCM model has formed the basis for evaluating and comparing the
potential benefits of mitigation measures designed to improve air quality,
which are then subjected to cost-benefit analysis. Examples of the
benefits to PM10 concentrations and annual costs and benefits of measures,
which may exceed £1 billion for individual measures, appear in Chapter 3
of the Updated Third Report of the Interdepartmental Group on Costs and
Benefits (Defra, 2007) [source 7].
- Implementation of abatement measures is key to the UK compliance with
EU Limit Values for PM10 [source 8]. Continued exceedence of the Limit
Values will lead to infraction proceedings being initiated by the European
Commission with subsequent imposition of large fines upon the UK. In 2011,
fines of up to £300 million were narrowly averted by a time extension
granted by the Commission. The PCM model was used to support a successful
application for a time extension to meet the PM10 Limit Value in London.
Sources to corroborate the impact
-
The Air Quality Strategy for England, Scotland, Wales and Northern
Ireland (Volume 1 and Volume 2), Cm 7169 NIA 61/06-07, July 2007.
- Williams, M., et al., Review of Air Quality Modelling in Defra, Report
to Defra, 7 April 2011, http://uk-air.defra.gov.uk/reports/cat20/1106290858_DefraModellingReviewFinalReport.pdf
- Corroborating statement from Principal Consultant and project manager
for UK Ambient Air Quality Assessment Contract, Ricardo-AEA, dated 19th
July 2013
- Corroborating statement from Head of Air Quality Evidence, Atmosphere
and Local Environment Programme, Defra, dated 29th July 2013
- UK Modelling under the Air Quality Directive (2008/50/EC) for 2009
Covering the following Air Quality Pollutants: SO2, NOx,
NO2, PM10, PM2.5, Lead, Benzene, CO and
Ozone, AEA Technology, Report No. AEAT/ENV/R/3069 Issue 1 (2010).
- UK Modelling under the Air Quality Directive (2008/50/EC) for 2010
Covering the following Air Quality Pollutants: SO2, NOx,
NO2, PM10, PM2.5, Lead, Benzene, CO and
Ozone, AEA Technology, Report No. AEAT/ENV/R/3215 Issue 1 (2011).
- An Economic Analysis to Inform the Air Quality Strategy, Update Report
of the Interdepartmental Group on Costs and Benefits, Defra, July 2007.
- Air Quality Expert Group (2005) Particulate Matter in the UK:
Summary. Defra, London.